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Characteristics of a novel nanosecond DBD microplasma reactor for flow applications

机译:用于流动的新型纳秒DBD微等离子体反应器的特性   应用

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摘要

We present a novel microplasma flow reactor using a dielectric barrierdischarge (DBD) driven by repetitively nanosecond high-voltage pulses. OurDBD-based geometry can generate a non-thermal plasma discharge at atmosphericpressure and below in a regular pattern of micro-channels. This reactor canwork continuously up to about 100 minutes in air, depending on pulse repetitionrate and operating pressure. We here present the geometry and the maincharacteristics of the reactor. Pulse energies of 1.9 $\mu$J and 2.7 $\mu$J perchannel at atmospheric pressure and 50 mbar, respectively, have been determinedby time-resolved measurements of current and voltage. Time-resolved opticalemission spectroscopy measurements have been performed to calculate therelative species concentrations and temperatures (vibrational and rotational)of the discharge. Effects of the operating pressure and the flow velocity onthe discharge intensity have been investigated. In addition, the effectivereduced electric field strength E/N has been obtained from the intensity ratioof vibronic emission bands of molecular nitrogen at different operatingpressures. The derived effective E/N increases gradually from 500 Td to 600 Tdwhen decreasing the pressure from one bar to 0.4 bar. Below 0.4 bar, furtherpressure reduction results in a significant increase in the effective E/N up toabout 2000 Td at 50 mbar.
机译:我们提出了一种新型的等离子流反应器,该反应器使用了介电势垒放电(DBD),由重复的纳秒高压脉冲驱动。基于DBD的几何结构可以在大气压及以下压力下以规则的微通道模式生成非热等离子体放电。该反应器可以在空气中连续工作约100分钟,具体取决于脉冲重复次数和工作压力。我们在这里介绍了反应堆的几何形状和主要特性。通过电流和电压的时间分辨测量,已确定在大气压和50 mbar下,每个通道的脉冲能量分别为1.9μJ和2.7μJ。已经进行了时间分辨的光发射光谱测量,以计算放电的相对物质浓度和温度(振动和旋转)。研究了工作压力和流速对放电强度的影响。另外,从不同工作压力下分子氮的电子发射带的强度比可以得到有效降低的电场强度E / N。当压力从1 bar降低到0.4 bar时,得出的有效E / N从500 Td逐渐增加到600 Td。低于0.4 bar,进一步降低压力会导致有效E / N显着提高,在50 mbar时高达2000 Td。

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